I have to say that even as a schoolchild neither the TOS Gorn nor the Horta were truly frightening.
I was watching monster movies on after school television, so the costumes for the Gorn and Horta were obviously that. I loved the Horta anyway.
The Gorn just seemed so inferior as compared to the Creature of the Black Lagoon and other contemporary examples. Time has only made the rubber suit more silly. In my view, the creature in TNG Conspiracy is falling into the same category now - memeable but not really scary.
But the Salt Monster I can agree was very disturbing. The fact that it was only shown briefly and there was no option for playback likely magnified it’s impact.
In terms of my own favourite, Andorians in Enterprise for the animatronics.